Substrate Diversity of L-Threonic Acid Dehydrogenase Homologs

Biochemistry (Mosc). 2020 Apr;85(4):463-471. doi: 10.1134/S0006297920040069.

Abstract

Despite physiological importance of aldonic sugar acids for living organisms, little is known about metabolic pathways of these compounds. Here, we investigated the functional diversity of homologs of L-threonic acid dehydrogenase (ThrDH; UniProt ID: Q0KBC7), an enzyme composed of two NAD-binding domains (PF14833 and PF03446). Ten ThrDH homologs with different genomic context were studied; seven new enzymatic activities were identified, such as (R)-pantoate dehydrogenase, L-altronic acid dehydrogenase, 6-deoxy-L-talonate dehydrogenase, L-idonic acid dehydrogenase, D-xylonic acid dehydrogenase, D-gluconic acid dehydrogenase, and 2-hydroxy-3-oxopantoate reductase activities. Two associated metabolic pathways were identified: L-idonic acid dehydrogenase was found to be involved in the degradation of L-idonic acid through oxidation/decarboxylation in Agrobacterium radiobacter K84, while 2-hydroxy-3-oxopantoate reductase was found to participate in D-glucarate catabolism through dehydration/cleavage in Ralstonia metallidurans CH34.

MeSH terms

  • Agrobacterium / enzymology*
  • Alcohol Oxidoreductases / classification
  • Alcohol Oxidoreductases / genetics
  • Alcohol Oxidoreductases / metabolism*
  • Amino Acid Sequence
  • Animals
  • Cupriavidus / enzymology*
  • Gluconates / metabolism
  • Humans
  • Isoenzymes
  • Metabolic Networks and Pathways*
  • Oxidation-Reduction
  • Sequence Homology
  • Substrate Specificity
  • Sugar Acids / metabolism
  • Xylose / analogs & derivatives
  • Xylose / metabolism

Substances

  • Gluconates
  • Isoenzymes
  • Sugar Acids
  • xylonic acid
  • idonic acid
  • altronic acid
  • Xylose
  • Alcohol Oxidoreductases
  • L-threonine 3-dehydrogenase
  • gluconic acid

Supplementary concepts

  • Cupriavidus metallidurans