A New Endoplasmic Reticulum (ER)-Targeting Fluorescent Probe for the Imaging of Cysteine in Living Cells

J Fluoresc. 2020 Dec;30(6):1357-1364. doi: 10.1007/s10895-020-02615-x. Epub 2020 Sep 1.

Abstract

Cysteine (Cys) is an important endogenous amino acid and plays critical physiological roles in living systems. Herein, an endoplasmic reticulum (ER)-targeting fluorescent probe (FER-Cys) was designed and prepared for imaging of Cys in living cells. The probe FER-Cys consists of a fluorescein framework as the fluorescent platform, acrylate group as the response site for the selective recognition of Cys, and ER-specific p-toluenesulfonamide fragment. After the response of probe FER-Cys to Cys, a turn-on fluorescence signal at 546 nm could be detected obviously. The probe FER-Cys further shows desirable selectivity to Cys. Finally, the probe FER-Cys was proven to selectively detect Cys in live cells and successfully image the changes of Cys level in the cell models of H2O2-induced redox imbalance.

Keywords: Endoplasmic reticulum-targeting; Fluorescent probe; Imaging of cysteine; Redox imbalance; Selective recognition.

MeSH terms

  • Cell Survival
  • Cysteine / metabolism*
  • Endoplasmic Reticulum / metabolism*
  • Fluorescent Dyes / chemistry
  • Fluorescent Dyes / metabolism*
  • HeLa Cells
  • Humans
  • Hydrogen Peroxide / pharmacology
  • Oxidation-Reduction / drug effects
  • Toluene / chemistry

Substances

  • Fluorescent Dyes
  • Toluene
  • Hydrogen Peroxide
  • Cysteine