Targeting PRC2 for the treatment of cancer: an updated patent review (2016 - 2020)

Expert Opin Ther Pat. 2021 Feb;31(2):119-135. doi: 10.1080/13543776.2021.1841167. Epub 2021 Jan 4.

Abstract

Introduction: PRC2 is a histone methyltransferase complex associated with several cancer types. Tazemetostat was recently approved as the first inhibitor targeting the catalytic subunit EZH2 and several other EZH2 inhibitors are now under clinical evaluation. Beyond EZH2, researchers have also explored other approaches including PRC2 activators, dual agents inhibiting both EZH1 and EZH2, allosteric inhibitors binding to EED, and compounds which induce the degradation of PRC2 constituent proteins.

Areas covered: This review provides an overview of anticancer therapies targeting PRC2 during the period 2016-2020 including clinical trials, patents and the scientific literature.

Expert opinion: The approval of tazemetostat marks the clinical validation of EZH2 for the treatment of cancer. Despite this success many questions remain; for instance, tazemetostat was briefly placed on clinical hold for safety concerns, while another EZH2 inhibitor (GSK126) demonstrated insufficient efficacy during a Phase I/II trial. It is important to understand these risks as PRC2 therapies progress through clinic evaluation. Alternative approaches to target PRC2 may offer distinct advantages over the inhibition of EZH2, including the potential to overcome EZH2 resistance mutations. However, these emerging modalities may also incur new challenges as they progress toward the clinic. Nonetheless, the diversity of agents under development represents a wealth of therapeutic options for future patients.

Keywords: EED; EZH2; PRC2; PROTACs; cancer; epigenetics; oncology.

Publication types

  • Review

MeSH terms

  • Animals
  • Antineoplastic Agents / pharmacology*
  • Benzamides / pharmacology
  • Biphenyl Compounds / pharmacology
  • Drug Resistance, Neoplasm / genetics
  • Enhancer of Zeste Homolog 2 Protein / antagonists & inhibitors
  • Enhancer of Zeste Homolog 2 Protein / genetics
  • Enhancer of Zeste Homolog 2 Protein / metabolism
  • Humans
  • Indoles / pharmacology
  • Molecular Targeted Therapy*
  • Morpholines / pharmacology
  • Mutation
  • Neoplasms / drug therapy*
  • Neoplasms / genetics
  • Neoplasms / pathology
  • Patents as Topic
  • Polycomb Repressive Complex 2 / metabolism
  • Pyridones / pharmacology

Substances

  • Antineoplastic Agents
  • Benzamides
  • Biphenyl Compounds
  • GSK-2816126
  • Indoles
  • Morpholines
  • Pyridones
  • EZH2 protein, human
  • Enhancer of Zeste Homolog 2 Protein
  • Polycomb Repressive Complex 2
  • tazemetostat