Aptamer-based proximity labeling guides covalent RNA modification

Chem Commun (Camb). 2021 Apr 11;57(28):3480-3483. doi: 10.1039/d1cc00786f. Epub 2021 Mar 10.

Abstract

We describe the development of a proximity-induced bio-orthogonal inverse electron demand Diels-Alder reaction that exploits the high-affinity interaction between a dienophile-modified RhoBAST aptamer and its tetramethyl rhodamine methyltetrazine substrate. We applied this concept for covalent RNA labeling in proof-of-principle experiments.

MeSH terms

  • Aptamers, Nucleotide / chemical synthesis
  • Aptamers, Nucleotide / chemistry*
  • Cycloaddition Reaction
  • Molecular Structure
  • RNA / chemistry*
  • Staining and Labeling*

Substances

  • Aptamers, Nucleotide
  • RNA