Leishmanial aspartyl-tRNA synthetase: Biochemical, biophysical and structural insights

Int J Biol Macromol. 2020 Dec 15;165(Pt B):2869-2885. doi: 10.1016/j.ijbiomac.2020.10.140. Epub 2020 Oct 22.

Abstract

Aminoacyl tRNA synthetases (aaRSs) are integral components of protein biosynthesis along with several non-canonical cellular processes. Inhibition studies of aaRSs presented these enzymes as promising drug targets in many pathogens, however aspartyl tRNA synthetase has not been studied in trypanosomatids despite its essentiality. Hence, full-length ORF of Leishmania donovani aspartyl tRNA synthetase (LdaspRS) was cloned and purified to homogeneity followed by molecular mass determination. The aminoacylation assay established that the purified protein performs its function optimally at physiological pH and temperature. The kinetic parameters of LdaspRS revealed the affinity of l-aspartate towards the enzyme to be very much lower than the cofactor. Our study also highlights the moonlighting function of LdaspRS to stimulate the pro-inflammatory cytokines and nitric oxide generation by host macrophage. Furthermore, CD and intrinsic tryptophan fluorescence measurements showed the changes in structural conformation at varying pH, denaturants and ligands. The modelled LdaspRS structure presented all the specific characteristics of class II aaRSs, while in silico study suggested binding of pyrimidine-derived inhibitors in its cofactor binding site with high affinity followed by validation using MD simulation. Altogether, this study could provide a platform for exploring LdaspRS to develop potential therapeutics against leishmaniasis.

Keywords: Aspartyl tRNA synthetase; Enzyme kinetics; Immunomodulation; Leishmania donovani; Pyrimidine-derived inhibitors; Structural characterization.

MeSH terms

  • Aminoacylation
  • Animals
  • Aspartate-tRNA Ligase / chemistry*
  • Aspartate-tRNA Ligase / genetics
  • Aspartate-tRNA Ligase / immunology
  • Aspartate-tRNA Ligase / metabolism*
  • Aspartic Acid / metabolism*
  • Cloning, Molecular
  • Evolution, Molecular
  • Humans
  • Hydrogen-Ion Concentration
  • Leishmania donovani / enzymology*
  • Leishmania donovani / genetics
  • Leishmania donovani / immunology
  • Mice
  • Models, Molecular
  • Nitric Oxide / metabolism
  • Open Reading Frames
  • Protein Conformation
  • Protozoan Proteins / chemistry
  • Protozoan Proteins / genetics
  • Protozoan Proteins / immunology
  • Protozoan Proteins / metabolism
  • Pyrimidines
  • RAW 264.7 Cells
  • THP-1 Cells
  • Temperature
  • Tryptophan / metabolism

Substances

  • Protozoan Proteins
  • Pyrimidines
  • Aspartic Acid
  • Nitric Oxide
  • Tryptophan
  • Aspartate-tRNA Ligase
  • pyrimidine