C-H and C-F coordination of arenes in neutral alkaline earth metal complexes

Dalton Trans. 2021 Jun 29;50(25):8685-8689. doi: 10.1039/d1dt01532j.

Abstract

A series of neutral magnesium and calcium complexes bearing an extremely bulky diamido ligand have been synthesised and crystallographically characterised. A number of these complexes feature rare group 2 metalaromatic interactions, such as the η6-coordination of benzene and 'agostic-like' C-H coordination, the latter previously unseen in neutral Mg and Ca complexes.