Mass spectrometry-based metabolomics: a guide for annotation, quantification and best reporting practices

Nat Methods. 2021 Jul;18(7):747-756. doi: 10.1038/s41592-021-01197-1. Epub 2021 Jul 8.

Abstract

Mass spectrometry-based metabolomics approaches can enable detection and quantification of many thousands of metabolite features simultaneously. However, compound identification and reliable quantification are greatly complicated owing to the chemical complexity and dynamic range of the metabolome. Simultaneous quantification of many metabolites within complex mixtures can additionally be complicated by ion suppression, fragmentation and the presence of isomers. Here we present guidelines covering sample preparation, replication and randomization, quantification, recovery and recombination, ion suppression and peak misidentification, as a means to enable high-quality reporting of liquid chromatography- and gas chromatography-mass spectrometry-based metabolomics-derived data.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Review

MeSH terms

  • Animals
  • Chromatography, Liquid
  • Gas Chromatography-Mass Spectrometry
  • Humans
  • Mass Spectrometry / methods*
  • Mass Spectrometry / standards
  • Metabolomics / methods*
  • Metabolomics / standards
  • Random Allocation
  • Specimen Handling
  • Workflow