HIPK2 phosphorylates HDAC3 for NF-κB acetylation to ameliorate colitis-associated colorectal carcinoma and sepsis

Proc Natl Acad Sci U S A. 2021 Jul 13;118(28):e2021798118. doi: 10.1073/pnas.2021798118.

Abstract

Although inflammation is critical for the clearance of pathogens, uncontrolled inflammation also contributes to the development of multiple diseases such as cancer and sepsis. Since NF-κB-mediated transactivation in the nucleus is pivotal downstream of various stimuli to induce inflammation, searching the nuclear-localized targets specifically regulating NF-κB activation will provide important therapeutic application. Here, we have identified that homeodomain-interacting protein kinase 2 (HIPK2), a nuclear serine/threonine kinase, increases its expression in inflammatory macrophages. Importantly, HIPK2 deficiency or overexpression could enhance or inhibit inflammatory responses in LPS-stimulated macrophages, respectively. HIPK2-deficient mice were more susceptible to LPS-induced endotoxemia and CLP-induced sepsis. Adoptive transfer of Hipk2+/- bone marrow cells (BMs) also aggravated AOM/DSS-induced colorectal cancer. Mechanistically, HIPK2 bound and phosphorylated histone deacetylase 3 (HDAC3) at serine 374 to inhibit its enzymatic activity, thus reducing the deacetylation of p65 at lysine 218 to suppress NF-κB activation. Notably, the HDAC3 inhibitors protected wild-type or Hipk2-/- BMs-reconstituted mice from LPS-induced endotoxemia. Our findings suggest that the HIPK2-HDAC3-p65 module in macrophages restrains excessive inflammation, which may represent a new layer of therapeutic mechanism for colitis-associated colorectal cancer and sepsis.

Keywords: HDAC3 phosphorylation; HIPK2; colon cancer; cytokine storm; p65 acetylation.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Acetylation
  • Animals
  • Cecum / pathology
  • Colitis / complications*
  • Colorectal Neoplasms / etiology*
  • Colorectal Neoplasms / metabolism
  • Cytokines / biosynthesis
  • Endotoxemia / complications
  • Histone Deacetylase Inhibitors / pharmacology
  • Histone Deacetylases / metabolism*
  • Humans
  • Inflammation / pathology
  • Inflammation Mediators / metabolism
  • Ligation
  • Lipopolysaccharides
  • Lysine / metabolism
  • Macrophages / metabolism
  • Macrophages / pathology
  • Mice
  • NF-kappa B / metabolism*
  • Phosphorylation / drug effects
  • Phosphoserine / metabolism
  • Protein Serine-Threonine Kinases / metabolism*
  • Punctures
  • Sepsis / etiology*
  • Sepsis / metabolism
  • Toll-Like Receptor 4 / metabolism
  • Toll-Like Receptor 9 / metabolism
  • Transcription Factor RelA / metabolism
  • Up-Regulation

Substances

  • Cytokines
  • Histone Deacetylase Inhibitors
  • Inflammation Mediators
  • Lipopolysaccharides
  • NF-kappa B
  • Toll-Like Receptor 4
  • Toll-Like Receptor 9
  • Transcription Factor RelA
  • Phosphoserine
  • Hipk2 protein, mouse
  • Protein Serine-Threonine Kinases
  • Histone Deacetylases
  • histone deacetylase 3
  • Lysine