Development of an orally delivered GLP-1 receptor agonist through peptide engineering and drug delivery to treat chronic disease

Sci Rep. 2021 Nov 18;11(1):22521. doi: 10.1038/s41598-021-01750-0.

Abstract

Peptide therapeutics are increasingly used in the treatment of disease, but their administration by injection reduces patient compliance and convenience, especially for chronic diseases. Thus, oral administration of a peptide therapeutic represents a significant advance in medicine, but is challenged by gastrointestinal instability and ineffective uptake into the circulation. Here, we have used glucagon-like peptide-1 (GLP-1) as a model peptide therapeutic for treating obesity-linked type 2 diabetes, a common chronic disease. We describe a comprehensive multidisciplinary approach leading to the development of MEDI7219, a GLP-1 receptor agonist (GLP-1RA) specifically engineered for oral delivery. Sites of protease/peptidase vulnerabilities in GLP-1 were removed by amino acid substitution and the peptide backbone was bis-lipidated to promote MEDI7219 reversible plasma protein binding without affecting potency. A combination of sodium chenodeoxycholate and propyl gallate was used to enhance bioavailability of MEDI7219 at the site of maximal gastrointestinal absorption, targeted by enteric-coated tablets. This synergistic approach resulted in MEDI7219 bioavailability of ~ 6% in dogs receiving oral tablets. In a dog model of obesity and insulin resistance, MEDI7219 oral tablets significantly decreased food intake, body weight and glucose excursions, validating the approach. This novel approach to the development of MEDI7219 provides a template for the development of other oral peptide therapeutics.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Administration, Oral
  • Animals
  • CHO Cells
  • Caco-2 Cells
  • Chemistry, Pharmaceutical / methods
  • Chenodeoxycholic Acid / administration & dosage
  • Chronic Disease* / drug therapy
  • Cricetinae
  • Cricetulus
  • Diabetes Mellitus, Type 2 / drug therapy
  • Drug Delivery Systems*
  • Drug Discovery
  • Glucagon-Like Peptide-1 Receptor* / agonists
  • Humans
  • Insulin-Secreting Cells / cytology
  • Male
  • Mice
  • Mice, Inbred C57BL
  • Peptides* / chemistry
  • Propyl Gallate / administration & dosage
  • Protein Engineering* / methods
  • Receptors, Glucagon / agonists
  • Tablets, Enteric-Coated

Substances

  • Chenodeoxycholic Acid
  • Glucagon-Like Peptide-1 Receptor
  • Peptides
  • Propyl Gallate
  • Receptors, Glucagon
  • Tablets, Enteric-Coated
  • MEDI7219