Bimetallic Au@Pt Nanocrystal Sensitization Mesoporous α-Fe2O3 Hollow Nanocubes for Highly Sensitive and Rapid Detection of Fish Freshness at Low Temperature

ACS Appl Mater Interfaces. 2021 Dec 8;13(48):57597-57608. doi: 10.1021/acsami.1c17695. Epub 2021 Nov 24.

Abstract

In this work, we present a new metal oxide semiconductor gas sensor for detecting trimethylamine (TMA) by bimetal Au@Pt-modified α-Fe2O3 hollow nanocubes (NCs) as sensing materials. The structure and morphological characteristics of Au@Pt/α-Fe2O3 were evaluated through multiple analyses, and their gas-sensitive performance was investigated. Compared with the pristine α-Fe2O3 NC sensor, the sensor based on Au@Pt/α-Fe2O3 NCs exhibited faster response time (5 s) and higher response (Ra/Rg = 32) toward 100 ppm TMA gas at a lower temperature (150 °C). Furthermore, we also assessed the Au@Pt/α-Fe2O3 NC sensor for detecting the freshness of Larimichthys crocea which have been observed by headspace solid-phase microextraction and gas chromatography-mass spectrometry. The high performance of the Au@Pt/α-Fe2O3 NCs is attributed to the special hollow morphology with a high specific surface area (212.9 m2/g) and the synergistic effect of the Au@Pt bimetal. The Au@Pt/α-Fe2O3 sensor shows promising application prospects in estimating seafood freshness on the spot.

Keywords: bimetallic nanocrystal; food freshness; gas sensing; trimethylamine; α-Fe2O3 nanocubes.

MeSH terms

  • Animals
  • Biomimetic Materials / chemistry*
  • Ferric Compounds / chemistry
  • Fish Products / analysis*
  • Fishes
  • Food Quality
  • Gold / chemistry
  • Materials Testing
  • Nanoparticles / chemistry*
  • Particle Size
  • Platinum / chemistry
  • Porosity
  • Surface Properties
  • Temperature*

Substances

  • Ferric Compounds
  • ferric oxide
  • Platinum
  • Gold