Polymeric dexamethasone prodrugs attenuate lupus nephritis in MRL/lpr mice with reduced glucocorticoid toxicity

Nanomedicine. 2022 Aug:44:102579. doi: 10.1016/j.nano.2022.102579. Epub 2022 Jun 26.

Abstract

Due to their potent immunosuppressive and anti-inflammatory effects, glucocorticoids (GCs) are the most widely used medications in treating lupus nephritis (LN). Long-term use of GCs, however, is associated with numerous off-target adverse effects. To reduce GCs' adverse effects, we previously developed two polymeric dexamethasone prodrug nanomedicines: N-(2-hydroxypropyl) methacrylamide (HPMA) copolymer-based dexamethasone prodrug (P-Dex), and micelle-forming polyethylene glycol (PEG)-based dexamethasone prodrug (ZSJ-0228). Both P-Dex and ZSJ-0228 provided sustained amelioration of LN in lupus-prone NZB/W F1 mice with reduced GC-associated adverse effects. Here, we have extended our investigation to the MRL/lpr mouse model of LN. Compared to dose equivalent daily dexamethasone sodium phosphate (Dex) treatment, monthly P-Dex or ZSJ-0228 treatments were more effective in reducing proteinuria and extending the lifespan of MRL/lpr mice. Unlike the daily Dex treatment, ZSJ-0228 was not associated with measurable GC-associated adverse effects. In contrast, adrenal gland atrophy was observed in P-Dex treated mice.

Keywords: Dexamethasone; Glucocorticoids; Lupus nephritis; Polymeric prodrug; Toxicity.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Animals
  • Dexamethasone / pharmacology
  • Dexamethasone / therapeutic use
  • Glucocorticoids / therapeutic use
  • Kidney
  • Lupus Nephritis* / drug therapy
  • Mice
  • Mice, Inbred MRL lpr
  • Mice, Inbred NZB
  • Polymers / pharmacology
  • Prodrugs* / pharmacology
  • Prodrugs* / therapeutic use

Substances

  • Glucocorticoids
  • Polymers
  • Prodrugs
  • Dexamethasone