A comprehensive review on reactive oxygen species (ROS) in advanced oxidation processes (AOPs)

Chencheng Dong; Wenzhang Fang; Qiuying Yi; Jinlong Zhang

doi:10.1016/j.chemosphere.2022.136205

A comprehensive review on reactive oxygen species (ROS) in advanced oxidation processes (AOPs)

Chemosphere. 2022 Dec;308(Pt 1):136205. doi: 10.1016/j.chemosphere.2022.136205. Epub 2022 Aug 29.

Authors

Chencheng Dong¹, Wenzhang Fang², Qiuying Yi³, Jinlong Zhang⁴

Affiliations

¹ Key Laboratory for Advanced Materials and Institute of Fine Chemicals, Shanghai Engineering Research Center for Multi-media Environmental Catalysis and Resource Utilization, School of Chemistry and Molecular Engineering, East China University of Science and Technology, 130 Meilong Road, Shanghai, 200237, PR China; Department of Civil Engineering, The University of Hong Kong, Hong Kong, China.
² MOE Key Laboratory of Macromolecular Synthesis and Functionalization, Department of Polymer Science and Engineering, Zhejiang University, Hangzhou, PR China.
³ State Key Laboratory of Pollution Control and Resource Reuse, Shanghai Institute of Pollution Control and Ecological Security, School of Environmental Science and Engineering, Tongji University, Shanghai, 200092, PR China.
⁴ Key Laboratory for Advanced Materials and Institute of Fine Chemicals, Shanghai Engineering Research Center for Multi-media Environmental Catalysis and Resource Utilization, School of Chemistry and Molecular Engineering, East China University of Science and Technology, 130 Meilong Road, Shanghai, 200237, PR China. Electronic address: [email protected].

PMID: 36049639
DOI: 10.1016/j.chemosphere.2022.136205

Abstract

In this account, the reactive oxygen species (ROS) were comprehensively reviewed, which were based on electro-Fenton and photo-Fenton processes and correlative membrane filtration technology. Specifically, this review focuses on the fundamental principles and applications of advanced oxidation processes (AOPs) based on a series of nanomaterials, and we compare the pros and cons of each method and point out the perspective. Further, the emerging reviews regarding AOPs rarely emphasize the involved ROS and consider the convenience of radical classification and transformation mechanism, such a review is of paramount importance to be needed. Owing to the strong oxidation ability of radical (e.g., •OH, O₂^•-, and SO₄^•-) and non-radical (e.g., ¹O₂ and H₂O₂), these ROS would attack the organic contaminants of emerging concern, thus achieving the goal of environmental remediation. Hopefully, this review can offer detailed theoretical guidance for the researchers, and we believe it able to offer the frontier knowledge of AOPs for wastewater treatment plants (WWTPs).

Keywords: AOP; Fenton; PMS; ROS; Singlet oxygen.

Publication types

Review

MeSH terms

Hydrogen Peroxide
Oxidation-Reduction
Reactive Oxygen Species
Water Pollutants, Chemical* / analysis
Water Purification* / methods

Substances

Reactive Oxygen Species
Water Pollutants, Chemical
Hydrogen Peroxide