Insights into olation reaction-driven coagulation and adsorption: A pathway for exploiting the surface properties of biochar

Sci Total Environ. 2023 Jan 1:854:158595. doi: 10.1016/j.scitotenv.2022.158595. Epub 2022 Sep 9.

Abstract

In this study, characterization of biochar for the efficient removal of cadmium was investigated. Biochar has a specific distribution of functional groups on its surface and has a natural electronegativity. Using carbonate as an olation reagent, the biochar coagulates with the olation reaction products. The maximum removal capacity reached 430.4 mg/g at pH = 4 (Langmuir Fit). Carbonate hydrolyzed on the surface of biochar, Cd2+ in solution undergoes olation with OH- and forms specially structured nanochains that are positively charged on the surface. The biochar with electronegativity on the surface coagulates with the cadmium hydroxide nanochains, and the cadmium-containing colloid formed by electrostatic attraction settles rapidly and removed. The biochar's re-flocculation performance was consistent, and the loadings could be changed to effectively remove cadmium while keeping the pH neutral at equilibrium.

Keywords: Adsorption; Biochar; Coagulation; Heavy metals; Olation reaction.

MeSH terms

  • Adsorption
  • Cadmium* / analysis
  • Carbonates
  • Charcoal / chemistry
  • Kinetics
  • Surface Properties
  • Water Pollutants, Chemical* / analysis

Substances

  • Cadmium
  • biochar
  • Charcoal
  • Carbonates
  • Water Pollutants, Chemical