P-450 HFLa, a form of cytochrome P-450 purified from human fetal livers, is the 16 alpha-hydroxylase of dehydroepiandrosterone 3-sulfate

J Biol Chem. 1987 Oct 5;262(28):13534-7.

Abstract

In a reconstituted system containing NADPH, dilauroyl-L-3-phosphatidylcholine, and NADPH-cytochrome P-450 reductase purified from rat liver microsomes, cytochrome P-450 (P-450 HFLa) purified from human fetal livers catalyzed the 16 alpha-hydroxylation of dehydroepiandrosterone 3-sulfate (DHEA-sulfate). Addition of cytochrome b5 purified from rat liver microsomes to the reconstituted system resulted in a remarkable increase in the hydroxylase activity. The level of P-450 HFLa in liver homogenates from human fetuses highly correlated with the activity of DHEA-sulfate 16 alpha-hydroxylase. Antibodies to P-450 HFLa inhibited the 16 alpha-hydroxylation of DHEA-sulfate in a dose-dependent manner. The NH2-terminal amino acid sequence of P-450 HFLa was similar to that of P-450NF (Beaune, P. H., Umbenhauer, D. R., Bork, R. W., Lloyd, R. S., and Guengerich, F. P. (1986) Proc. Natl. Acad. Sci. U. S. A. 83, 8064-8068). We conclude that P-450 HFLa is a form of cytochrome P-450 involved in the 16 alpha-hydroxylation of DHEA-sulfate.

MeSH terms

  • Amino Acid Sequence
  • Antigen-Antibody Complex
  • Aryl Hydrocarbon Hydroxylases*
  • Cytochrome P-450 CYP2C8
  • Cytochrome P-450 CYP2C9
  • Cytochrome P-450 Enzyme System / metabolism*
  • Cytochrome P450 Family 2
  • Cytochrome b Group / metabolism
  • Cytochromes b5
  • Fetus
  • Gas Chromatography-Mass Spectrometry
  • Humans
  • Immunoglobulin G
  • Kinetics
  • Liver / embryology
  • Liver / enzymology*
  • Steroid 16-alpha-Hydroxylase*

Substances

  • Antigen-Antibody Complex
  • Cytochrome b Group
  • Immunoglobulin G
  • Cytochromes b5
  • Cytochrome P-450 Enzyme System
  • CYP2C9 protein, human
  • Cytochrome P-450 CYP2C9
  • Aryl Hydrocarbon Hydroxylases
  • CYP2C11 protein, rat
  • CYP2C8 protein, human
  • Cytochrome P-450 CYP2C8
  • Cytochrome P450 Family 2
  • Steroid 16-alpha-Hydroxylase