Repurposing amine and carboxylic acid building blocks with an automatable esterification reaction

Chem Commun (Camb). 2023 Jan 24;59(8):1026-1029. doi: 10.1039/d2cc05670d.

Abstract

New methodologies to unite amines and carboxylic acids that complement the popular amide coupling can significantly expand accessible chemical space if they yield products distinct from the classic R-NHC(O)-R' amide arrangement. Here we have developed an amine-acid esterification reaction based on pyridinium salt activation of amine C-N bonds to create products of type R-OC(O)-R' upon reaction with alkyl and aryl carboxylic acids. The protocol is robust and facile as demonstrated by automation on open-source robotics.

MeSH terms

  • Amides / chemistry
  • Amines* / chemistry
  • Carboxylic Acids* / chemistry
  • Esterification

Substances

  • Amines
  • Carboxylic Acids
  • Amides