Reaction of 5'-p-fluorosulfonylbenzoyladenosine with the catalytic and AMP allosteric sites of microsomal HMG-CoA reductase kinase

Biochem Biophys Res Commun. 1987 Nov 13;148(3):1009-16. doi: 10.1016/s0006-291x(87)80232-2.

Abstract

The nucleotide analogue 5-p-fluorosulfonylbenzoyladenosine reacts with rat liver microsomal 3-hydroxy-3-methylglutaryl-CoA reductase kinase, causing a rapid loss of the AMP activation capacity and a slower inactivation of the catalytic activity. The rate constant for loss of AMP activation is eleven times higher (K1 = 0.107 min-1) than the rate constant for inactivation (K2 = 0.0094 min-1). Mg-ATP protects preferentially against inactivation, while Mg-AMP at a low concentration (7.5/0.05 mM) protects preferentially against loss of the AMP activation capacity. Oppositely, Mg-ADP at a low concentration (7.5/0.05 mM) hardly protects against loss of AMP activation capacity. We conclude that microsomal reductase kinase has distinct sites for activation and catalysis.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • AMP-Activated Protein Kinases
  • Adenosine / analogs & derivatives*
  • Adenosine / metabolism
  • Adenosine Monophosphate / metabolism
  • Adenosine Triphosphate / metabolism
  • Allosteric Regulation
  • Animals
  • Binding Sites
  • Binding, Competitive
  • Kinetics
  • Magnesium / metabolism
  • Microsomes, Liver / enzymology*
  • Multienzyme Complexes / metabolism*
  • Protein Kinases / metabolism*
  • Protein Serine-Threonine Kinases*
  • Rats

Substances

  • Multienzyme Complexes
  • Adenosine Monophosphate
  • 5'-(4-fluorosulfonylbenzoyl)adenosine
  • Adenosine Triphosphate
  • Protein Kinases
  • Protein Serine-Threonine Kinases
  • AMP-Activated Protein Kinases
  • Magnesium
  • Adenosine