Total Synthesis and Absolute Configuration Determination of the α-Glycosidase Inhibitor (3 S,4 R)-6-Acetyl-3-hydroxy-2,2-dimethylchroman-4-yl (Z)-2-Methylbut-2-enoate from Ageratina grandifolia

J Nat Prod. 2023 Jul 28;86(7):1878-1883. doi: 10.1021/acs.jnatprod.3c00236. Epub 2023 Jun 14.

Abstract

Herein, we report the first total synthesis of α-glycosidase inhibitor (3R, 4S)-6-acetyl-3-hydroxy-2,2-dimethylchroman-4-yl (Z)-2-methylbut-2-enoate as well as its enantiomer. Our synthesis confirms the chromane structure separately proposed by Navarro-Vazquez and Mata, on the basis of DFT computations. Furthermore, our synthesis allowed us to determine the absolute configuration of the natural compound as (3S, 4R) and not (3R, 4S).

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Ageratina*
  • Glycoside Hydrolases
  • Molecular Structure
  • Stereoisomerism

Substances

  • Glycoside Hydrolases