Potent nitric oxide inhibitory sesquiterpenoids from the rhizome of Curcuma aromatica Salisb

Nat Prod Res. 2024 May;38(10):1739-1747. doi: 10.1080/14786419.2023.2222219. Epub 2023 Jun 15.

Abstract

One new sesquiterpenoid, curcaromatin (1), together with twenty-one known compounds 2-22, were isolated from the rhizomes of Curcuma aromatica Salisb. (Zingiberaceae). Their structures were established by extensive spectroscopic (1D and 2D NMR and HR-MS) analysis. Most of the isolated compounds were investigated for nitric oxide (NO) production in lipopolysaccharide (LPS)-activated RAW264.7 cells. (-)-Xanthorrhizol (3) displayed the strongest NO inhibitory activity with an IC50 value of 4.3 μM, which was 3.7-fold more active than the reference compound, aminoguanidine (IC50 15.9 μM). The selectivity index (SI > 28.1) of compound 3 was almost 3-fold higher than that of aminoguanidine.

Keywords: Curcuma aromatica; Zingiberaceae; anti-inflammation; nitric oxide inhibitory activity; sesquiterpenoids.

MeSH terms

  • Curcuma* / chemistry
  • Guanidines*
  • Lipopolysaccharides / pharmacology
  • Molecular Structure
  • Nitric Oxide
  • Rhizome / chemistry
  • Sesquiterpenes* / chemistry

Substances

  • pimagedine
  • Nitric Oxide
  • Sesquiterpenes
  • Lipopolysaccharides
  • Guanidines