Combined inhibition of pyruvate dehydrogenase kinase 1 and lactate dehydrogenase a induces metabolic and signaling reprogramming and enhances lung adenocarcinoma cell killing

Cancer Lett. 2023 Nov 28:577:216425. doi: 10.1016/j.canlet.2023.216425. Epub 2023 Oct 5.

Abstract

Lung adenocarcinoma (LUAD) is one of the most prevalent and aggressive types of lung cancer. Metabolic reprogramming plays a critical role in the development and progression of LUAD. Pyruvate dehydrogenase kinase 1 (PDK1) and lactate dehydrogenase A (LDHA) are two key enzymes involved in glucose metabolism, whilst their aberrant expressions are often associated with tumorigenesis. Herein, we investigated the anticancer effects of combined inhibition of PDK1 and LDHA in LUAD in vitro and in vivo and its underlying mechanisms of action. The combination of a PDK1 inhibitor, 64, and a LDHA inhibitor, NHI-Glc-2, led to a synergistic growth inhibition in 3 different LUAD cell lines and more than additively suppressed tumor growth in the LUAD xenograft H1975 model. This combination also inhibited cellular migration and colony formation, while it induced a metabolic shift from glycolysis to oxidative phosphorylation (OXPHOS) resulting in mitochondrial depolarization and apoptosis in LUAD cells. These effects were related to modulation of multiple cell signaling pathways, including AMPK, RAS/ERK, and AKT/mTOR. Our findings demonstrate that simultaneous inhibition of multiple glycolytic enzymes (PDK1 and LDHA) is a promising novel therapeutic approach for LUAD.

Keywords: Anticancer; Combination treatment; Non-small cell lung cancer; Warburg effect.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adenocarcinoma of Lung* / drug therapy
  • Cell Death
  • Cell Line, Tumor
  • Cell Proliferation
  • Glycolysis
  • Humans
  • L-Lactate Dehydrogenase
  • Lactate Dehydrogenase 5* / antagonists & inhibitors
  • Lactate Dehydrogenase 5* / metabolism
  • Lung Neoplasms* / drug therapy
  • Lung Neoplasms* / genetics
  • Pyruvate Dehydrogenase Acetyl-Transferring Kinase* / antagonists & inhibitors
  • Pyruvate Dehydrogenase Acetyl-Transferring Kinase* / metabolism
  • Signal Transduction

Substances

  • L-Lactate Dehydrogenase
  • Lactate Dehydrogenase 5
  • Pyruvate Dehydrogenase Acetyl-Transferring Kinase