Proteomics analysis of histone deacetylase inhibitor-resistant solid tumors reveals resistant signatures and potential drug combinations

Acta Pharmacol Sin. 2024 Jun;45(6):1305-1315. doi: 10.1038/s41401-024-01236-5. Epub 2024 Feb 21.

Abstract

Histone deacetylase inhibitors (HDACis) are important drugs for cancer therapy, but the indistinct resistant mechanisms of solid tumor therapy greatly limit their clinical application. In this study we conducted HDACi-perturbated proteomics and phosphoproteomics analyses in HDACi-sensitive and -resistant cell lines using a tandem mass tag (TMT)-based quantitative proteomic strategy. We found that the ribosome biogenesis proteins MRTO4, PES1, WDR74 and NOP16 vital to tumorigenesis might regulate the tumor sensitivity to HDACi. By integrating HDACi-perturbated protein signature with previously reported proteomics and drug sensitivity data, we predicted and validated a series of drug combination pairs potentially to enhance the sensitivity of HDACi in diverse solid tumor. Functional phosphoproteomic analysis further identified the kinase PDK1 and ROCK as potential HDACi-resistant signatures. Overall, this study reveals the potential HDACi-resistant signatures and may provide promising drug combination strategies to attenuate the resistance of solid tumor to HDACi.

Keywords: drug resistance; histone deacetylase inhibitor; proteomics; solid tumor; vorinostat (SAHA).

MeSH terms

  • Antineoplastic Agents / pharmacology
  • Antineoplastic Agents / therapeutic use
  • Cell Line, Tumor
  • Drug Resistance, Neoplasm* / drug effects
  • Histone Deacetylase Inhibitors* / pharmacology
  • Humans
  • Neoplasms* / drug therapy
  • Neoplasms* / metabolism
  • Proteomics*

Substances

  • Histone Deacetylase Inhibitors
  • Antineoplastic Agents