Upregulation of Hepatic Glutathione S-Transferase Alpha 1 Ameliorates Metabolic Dysfunction-Associated Steatosis by Degrading Fatty Acid Binding Protein 1

Int J Mol Sci. 2024 May 7;25(10):5086. doi: 10.3390/ijms25105086.

Abstract

Metabolic dysfunction-associated steatotic liver disease (MASLD) is the most common metabolic disease of the liver, characterized by hepatic steatosis in more than 5% of hepatocytes. However, despite the recent approval of the first drug, resmetirom, for the management of metabolic dysfunction-associated steatohepatitis, decades of target exploration and hundreds of clinical trials have failed, highlighting the urgent need to find new druggable targets for the discovery of innovative drug candidates against MASLD. Here, we found that glutathione S-transferase alpha 1 (GSTA1) expression was negatively associated with lipid droplet accumulation in vitro and in vivo. Overexpression of GSTA1 significantly attenuated oleic acid-induced steatosis in hepatocytes or high-fat diet-induced steatosis in the mouse liver. The hepatoprotective and anti-inflammatory drug bicyclol also attenuated steatosis by upregulating GSTA1 expression. A detailed mechanism showed that GSTA1 directly interacts with fatty acid binding protein 1 (FABP1) and facilitates the degradation of FABP1, thereby inhibiting intracellular triglyceride synthesis by impeding the uptake and transportation of free fatty acids. Conclusion: GSTA1 may be a good target for the discovery of innovative drug candidates as GSTA1 stabilizers or enhancers against MASLD.

Keywords: bicyclol; drug target; fatty acid binding protein 1; glutathione S-transferase alpha 1; hepatic steatosis.

MeSH terms

  • Animals
  • Diet, High-Fat / adverse effects
  • Fatty Acid-Binding Proteins* / genetics
  • Fatty Acid-Binding Proteins* / metabolism
  • Fatty Liver* / drug therapy
  • Fatty Liver* / metabolism
  • Glutathione Transferase* / genetics
  • Glutathione Transferase* / metabolism
  • Hep G2 Cells
  • Hepatocytes / drug effects
  • Hepatocytes / metabolism
  • Humans
  • Isoenzymes
  • Lipid Metabolism / drug effects
  • Liver / drug effects
  • Liver / metabolism
  • Liver / pathology
  • Male
  • Mice
  • Mice, Inbred C57BL
  • Oleic Acid / metabolism
  • Triglycerides / metabolism
  • Up-Regulation* / drug effects

Substances

  • Glutathione Transferase
  • Fatty Acid-Binding Proteins
  • GSTA1 protein, human
  • Oleic Acid
  • Triglycerides
  • FABP1 protein, human
  • glutathione S-transferase alpha
  • Isoenzymes