Optimizing extraction methods by a comprehensive experimental approach and characterizing polyphenol compositions of Ecklonia radiata

Food Chem. 2024 Oct 15:455:139926. doi: 10.1016/j.foodchem.2024.139926. Epub 2024 May 31.

Abstract

Brown seaweed Ecklonia radiata harbors valuable polyphenols, notably phlorotannins, prized for their health benefits. This study optimized phlorotannin extraction via conventional solvent extraction and ultrasound-assisted extraction methods, utilizing variable concentrations of ethanol. Employing fractional factorial designs, key variables were identified. Steepest ascent/descent method and central composite rotatable designs refined optimal conditions, enhancing phlorotannin and polyphenol yields, and antioxidant capacities. Under optimized conditions, phlorotannin contents reached 2.366 ± 0.01 and 2.596 ± 0.04 PGE mg/g, total polyphenol contents peaked at 10.223 ± 0.03 and 10.836 ± 0.02 GAE mg/g. Robust antioxidant activity was observed: DPPH and OH radical scavenging capacities measured 27.891 ± 0.06 and 17.441 ± 0.08 TE mg/g, and 37.498 ± 1.12 and 49.391 ± 0.82 TE mg/g, respectively. Reducing power capacities surged to 9.016 ± 0.02 and 28.110 ± 0.10 TE mg/g. Liquid chromatography-mass spectrometry (LC-MS) and high-performance liquid chromatography (HPLC) analyses revealed enriched antioxidant compounds. Variations in polyphenol profiles were noted, potentially influencing antioxidant capacity nuances. This study illuminated the potential of E. radiata potential as a polyphenol source and offers optimized extraction methods poised to benefit various industries.

Keywords: Antioxidant; Ecklonia radiata; Optimization; Phlorotannins; Ultrasound-assisted extraction.

Publication types

  • Evaluation Study

MeSH terms

  • Antioxidants* / chemistry
  • Antioxidants* / isolation & purification
  • Chemical Fractionation / methods
  • Chromatography, High Pressure Liquid
  • Mass Spectrometry
  • Phaeophyceae / chemistry
  • Plant Extracts / chemistry
  • Plant Extracts / isolation & purification
  • Polyphenols* / analysis
  • Polyphenols* / chemistry
  • Polyphenols* / isolation & purification
  • Seaweed* / chemistry
  • Zygophyllaceae / chemistry

Substances

  • Polyphenols
  • Antioxidants
  • Plant Extracts