Talaesthanes A-C, three new meroterpenoids from the endophytic fungus Talaromyces primulinus H21

Fitoterapia. 2024 Sep:177:106085. doi: 10.1016/j.fitote.2024.106085. Epub 2024 Jun 18.

Abstract

Three new meroterpenoids (1-3) and ten known ones (4-13) were obtained from the endophytic fungus Talaromyces primulinus H21 isolated from the plant of Euphorbia sikkimensis. Their structures including their absolute configurations were elucidated by extensive analysis of spectroscopic data such as HR-ESI-MS, 1D/2D NMR, and X-ray diffraction of single crystal together with comparison of experimental ECD with calculated ECD. All compounds were examined for their inhibitory effects on nitric oxide (NO) production induced by lipopolysaccharide (LPS) in RAW264.7 cells, and compounds 3, 9, 12, and 13 exhibited certain inhibition on NO production, with IC50 values of 27.19, 41.55, 25.23, and 24.71 μM, respectively.

Keywords: Anti-inflammatory activity; Endophytic fungus; Meroterpenoids; Talaromyces primulinus.

MeSH terms

  • Animals
  • China
  • Endophytes / chemistry
  • Mice
  • Molecular Structure
  • Nitric Oxide* / metabolism
  • RAW 264.7 Cells
  • Talaromyces* / chemistry
  • Terpenes* / isolation & purification
  • Terpenes* / pharmacology

Substances

  • Nitric Oxide
  • Terpenes