Leveraging a self-cleaving peptide for tailored control in proximity labeling proteomics

Cell Rep Methods. 2024 Jul 15;4(7):100818. doi: 10.1016/j.crmeth.2024.100818. Epub 2024 Jul 9.

Abstract

Protein-protein interactions play an important biological role in every aspect of cellular homeostasis and functioning. Proximity labeling mass spectrometry-based proteomics overcomes challenges typically associated with other methods and has quickly become the current state of the art in the field. Nevertheless, tight control of proximity-labeling enzymatic activity and expression levels is crucial to accurately identify protein interactors. Here, we leverage a T2A self-cleaving peptide and a non-cleaving mutant to accommodate the protein of interest in the experimental and control TurboID setup. To allow easy and streamlined plasmid assembly, we built a Golden Gate modular cloning system to generate plasmids for transient expression and stable integration. To highlight our T2A Split/link design, we applied it to identify protein interactions of the glucocorticoid receptor and severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2) nucleocapsid and non-structural protein 7 (NSP7) proteins by TurboID proximity labeling. Our results demonstrate that our T2A split/link provides an opportune control that builds upon previously established control requirements in the field.

Keywords: CP: Biotechnology; Golden Gate assembly; T2A peptide; T2A split/link; TurboID; glucocorticoid receptor; interactomics; non-structural protein 7; nucleocapsid protein; proteomics; proximity labeling.

MeSH terms

  • COVID-19 / metabolism
  • COVID-19 / virology
  • Coronavirus Nucleocapsid Proteins / chemistry
  • Coronavirus Nucleocapsid Proteins / genetics
  • Coronavirus Nucleocapsid Proteins / metabolism
  • HEK293 Cells
  • Humans
  • Mass Spectrometry / methods
  • Peptides* / chemistry
  • Peptides* / metabolism
  • Phosphoproteins / genetics
  • Phosphoproteins / metabolism
  • Plasmids / genetics
  • Plasmids / metabolism
  • Protein Interaction Mapping / methods
  • Proteomics* / methods
  • Receptors, Glucocorticoid / chemistry
  • Receptors, Glucocorticoid / genetics
  • Receptors, Glucocorticoid / metabolism
  • SARS-CoV-2* / genetics
  • SARS-CoV-2* / metabolism

Substances

  • Peptides
  • Receptors, Glucocorticoid
  • Coronavirus Nucleocapsid Proteins
  • nucleocapsid phosphoprotein, SARS-CoV-2
  • Phosphoproteins