Injectable dual thermoreversible hydrogel for sustained intramuscular drug delivery

J Control Release. 2024 Oct:374:590-605. doi: 10.1016/j.jconrel.2024.08.034. Epub 2024 Aug 30.

Abstract

Herein, we reported novel docetaxel-decorated solid lipid nanoparticle (DCT-SLN)-loaded dual thermoreversible system (DCT-DRTS) for intramuscular administration with reduced burst effect, sustained release and improved antitumor efficacy. The optimized DCT-DRTs was subjected to in-vitro and in-vivo analyses. Antitumor evaluation of the DCT-DRTS was executed and compared with DCT-hydrogel, and DCT-suspension trailed by the histopathological and immune-histochemical analyses. The DCT-SLN gave a mean particle size of 157 nm and entrapment efficiency of 93 %. It was a solid at room temperature, and changed to liquid at physiological temperature due to its melting point of about 32 °C. Unlikely, poloxamer mixture remained liquefied at 25-27 °C, however converted to gel at physiological temperature. This behavior demonstrated opposed reversible property of the DCT-SLN and poloxamer hydrogel in DCT-DRTS system, making it ideal for intramuscular administration and quick gelation inside the body. The DCT-DRTS sustained the drugs release and unlike DCT-hydrogel, the preliminary plasma concentration of DCT-DRTS was significantly reduced, overcoming the burst release. A meaningfully enhanced antitumor efficacy and improved survival rate was observed from DCT-DRTS in tumor cell xenograft athymic nude mice. Additionally, increased apoptotic and reduced proliferation markers were observed in DCT-DRTS treated tumor masses. It was concluded that DCT-DRTS may be a suitable choice for intramuscular administration of DCT with sustained release, improved bioavailability, reduced toxicity and enhanced antitumor effects.

Keywords: Bioavailability; Burst effect; Docetaxel; Dual thermoreversible system; Solid lipid nanoparticles; Sustained release; Tumor.

MeSH terms

  • Animals
  • Antineoplastic Agents* / administration & dosage
  • Antineoplastic Agents* / pharmacokinetics
  • Cell Line, Tumor
  • Delayed-Action Preparations* / chemistry
  • Docetaxel* / administration & dosage
  • Docetaxel* / pharmacokinetics
  • Drug Carriers / chemistry
  • Drug Delivery Systems
  • Drug Liberation
  • Female
  • Humans
  • Hydrogels* / administration & dosage
  • Hydrogels* / chemistry
  • Injections, Intramuscular
  • Lipids / administration & dosage
  • Lipids / chemistry
  • Liposomes
  • Male
  • Mice
  • Mice, Inbred BALB C
  • Mice, Nude
  • Nanoparticles* / administration & dosage
  • Nanoparticles* / chemistry
  • Neoplasms / drug therapy
  • Poloxamer / chemistry
  • Taxoids / administration & dosage
  • Taxoids / chemistry
  • Taxoids / pharmacokinetics
  • Temperature

Substances

  • Hydrogels
  • Antineoplastic Agents
  • Docetaxel
  • Delayed-Action Preparations
  • Poloxamer
  • Lipid Nanoparticles
  • Lipids
  • Drug Carriers
  • Taxoids
  • Liposomes