Degradation of poly(3-hydroxybutyrate) by poly(3-hydroxybutyrate) depolymerase from Alcaligenes faecalis T1

Biochim Biophys Acta. 1986 Jan 15;880(1):46-53. doi: 10.1016/0304-4165(86)90118-2.

Abstract

The extracellular poly(3-hydroxybutyrate) depolymerase purified from Alcaligenes faecalis T1 has two disulfide bonds, one of which appears to be necessary for the full enzyme activity. This depolymerase hydrolyzed not only hydrophobic poly(3-hydroxybutyrate) but also water-soluble trimer and larger oligomers of D-(-)-3-hydroxybutyrate, regardless of their solubilities in water. Kinetic analyses with oligomers of various sizes indicated that the substrate cleaving site of the enzyme consisted of four subsites with individual affinities for monomer units of the substrate. Analyses of the hydrolytic products of oligomers, which had labeled D-(-)-3-hydroxybutyrate at the hydroxy terminus, showed that the enzyme cleaved only the second ester linkage from the hydroxy terminus of the trimer and tetramer, and acted as an endo-type hydrolase toward the pentamer and higher oligomers. The enzyme appeared to have a hydrophobic site which interacted with poly(3-hydroxybutyrate) and determined the affinity of the enzyme toward the hydrophobic substrate.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Alcaligenes / enzymology*
  • Carboxylic Ester Hydrolases / antagonists & inhibitors
  • Carboxylic Ester Hydrolases / metabolism*
  • Hydroxybutyrates / metabolism
  • Kinetics
  • Organosilicon Compounds*
  • Polyesters*
  • Polyethylene Glycols / pharmacology
  • Polymers / metabolism
  • Silicon / pharmacology
  • Structure-Activity Relationship
  • Substrate Specificity
  • Sulfhydryl Compounds / pharmacology
  • Sulfhydryl Reagents / pharmacology

Substances

  • Hydroxybutyrates
  • Organosilicon Compounds
  • Polyesters
  • Polymers
  • Sulfhydryl Compounds
  • Sulfhydryl Reagents
  • t-butyldimethylsilyl compounds
  • poly-beta-hydroxybutyrate
  • Polyethylene Glycols
  • Carboxylic Ester Hydrolases
  • poly-beta-hydroxybutyrate depolymerase
  • Silicon