Enhanced field emission performance of gold nanoparticle decorated Bi2S3 nanoflowers

Nanoscale Adv. 2024 Nov 13;7(1):310-319. doi: 10.1039/d4na00539b. eCollection 2024 Dec 17.

Abstract

Au nanoparticles (NPs) are decorated on hydrothermally synthesized Bi2S3 nanorods (NRs) to enhance the field electron emission (FEE) performance as compared to bare Bi2S3 nanorods, resulting in reduction in turn-on field from 3.7 to 2.7 V μm-1 (at the current density of 1.0 μA cm-2) with significant increment in maximum emission current density from 138 to 604.8 μA cm-2 (at a field of 7.8 V μm-1) respectively. FESEM/TEM reveals that Bi2S3 nanoflowers are assembled from Bi2S3 NRs of a typical diameter of 120 ± 10 nm, and Au NPs of diameter about 5-10 nm are uniformly decorated onto the surface of NRs to form an Au/Bi2S3 composite. XRD analysis suggests that the as-synthesized product consists of orthorhombic Bi2S3 NRs decorated with face-centered cubic Au NPs. The XPS spectrum shows the elemental mapping of the as-synthesized Au/Bi2S3. Improvement in field emission properties is mainly attributed to a reduction in work function and increasing emitting sites due to Au NP decoration.