Microbial-derived bile acid reverses inflammation in IBD via GPBAR1 agonism and RORγt inverse agonism

Biomed Pharmacother. 2024 Dec:181:117731. doi: 10.1016/j.biopha.2024.117731. Epub 2024 Dec 9.

Abstract

The interplay between the dysbiotic microbiota and bile acids is a critical determinant for development of a dysregulated immune system in inflammatory bowel disease (IBD). Here we have investigated the fecal bile acid metabolome, gut microbiota composition, and immune responses in IBD patients and murine models of colitis and found that IBD associates with an elevated excretion of primary bile acids while secondary, allo- and oxo- bile acids were reduced. These changes correlated with the disease severity, mucosal expression of pro-inflammatory cytokines and chemokines, and reduced inflow of anti-inflammatory macrophages and Treg in the gut. Analysis of bile acids metabolome in the feces allowed the identification of five bile acids: 3-oxo-DCA, 3-oxo-LCA, allo-LCA, iso-allo-LCA and 3-oxo-UDCA, whose excretion was selectively decreased in IBD patients and diseased mice. By transactivation assay and docking calculations all five bile acids were shown to act as GPBAR1 agonists and RORγt inverse agonists, skewing Th17/Treg ratio and macrophage polarization toward an M2 phenotype. In a murine model of colitis, administration of 3-oxo-DCA suffices to reverse colitis development and intestinal dysbiosis in a GPBAR1-dependent manner. In vivo administration of 3-oxo-DCA to colitic mice also reverses disease severity and RORγt activation induced by a RORγt agonist and IL-23, a Th17 inducing cytokine. These results demonstrated that intestinal excretion of 3-oxoDCA, a dual GPBAR1 agonist and RORγt inverse agonist, is reduced in IBD and in models of colitis and its restitution protects against colitis development, highlighting a potential role for this agent in IBD management.

Keywords: 3-oxo-DCA; Bile acids; GPBAR1; Gut microbiota; Inflammatory bowel disease; RORγt.

MeSH terms

  • Adult
  • Animals
  • Bile Acids and Salts* / metabolism
  • Colitis* / drug therapy
  • Colitis* / metabolism
  • Colitis* / microbiology
  • Disease Models, Animal
  • Feces / chemistry
  • Feces / microbiology
  • Female
  • Gastrointestinal Microbiome* / drug effects
  • Humans
  • Inflammation / drug therapy
  • Inflammation / metabolism
  • Inflammatory Bowel Diseases* / drug therapy
  • Inflammatory Bowel Diseases* / metabolism
  • Inflammatory Bowel Diseases* / microbiology
  • Macrophages / drug effects
  • Macrophages / metabolism
  • Male
  • Mice
  • Mice, Inbred C57BL*
  • Middle Aged
  • Nuclear Receptor Subfamily 1, Group F, Member 3* / metabolism
  • Receptors, G-Protein-Coupled* / agonists
  • Receptors, G-Protein-Coupled* / metabolism

Substances

  • Bile Acids and Salts
  • Nuclear Receptor Subfamily 1, Group F, Member 3
  • GPBAR1 protein, human
  • Receptors, G-Protein-Coupled
  • Gpbar1 protein, mouse