Revealing the Anticancer Mechanism of Cephaibol A, a Peptaibol Isolated from Acremonium tubakii BMC-58, Triggering Apoptosis via the Mitochondrial Pathway in Human Breast Cancer Cells

Biol Pharm Bull. 2024;47(12):2065-2075. doi: 10.1248/bpb.b24-00537.

Abstract

Cephaibol A was isolated from a freshwater fungus Acremonium tubakii BMC-58 extract which composed of 16 amino acids and featuring multiple α-aminoisobutyric acid. We investigated the cytotoxicity of cephaibol A on MDA-MB-231 cells to elucidate its potential antitumor activity and mechanism. The study found that cephaibol A concentration-dependently blocked the cell cycle in S phase and inhibited cell proliferation. Meanwhile, cephaibol A could reduce the migration and invasion abilities of MDA-MB-231 cells. Further studies proved that cephaibol A caused mitochondrial dysfunction and increased reactive oxygen species (ROS) accumulation. Mitochondrial membrane potential (ΔΨm) assay suggested that cephaibol A induced apoptosis by affecting Bcl-2, Bax and cytochrome c levels, thus decreasing ΔΨm and activating the caspase cascade reaction. Moreover, cephaibol A significantly inhibited tumor growth and improved survival rates in the MDA-MB-231 cell mice model. These findings established cephaibol A as a potential antitumor agent that inhibited tumor cell proliferation in vitro and in vivo by affecting mitochondrial dysfunction and inducing apoptosis in MDA-MB-231 cells through structural damage.

Keywords: apoptosis; cephaibol A; mitochondria; natural product; triple-negative breast cancer.

MeSH terms

  • Acremonium*
  • Animals
  • Antineoplastic Agents* / isolation & purification
  • Antineoplastic Agents* / pharmacology
  • Antineoplastic Agents* / therapeutic use
  • Apoptosis* / drug effects
  • Breast Neoplasms* / drug therapy
  • Breast Neoplasms* / pathology
  • Cell Line, Tumor
  • Cell Movement / drug effects
  • Cell Proliferation* / drug effects
  • Female
  • Humans
  • Membrane Potential, Mitochondrial* / drug effects
  • Mice
  • Mice, Inbred BALB C
  • Mice, Nude
  • Mitochondria* / drug effects
  • Mitochondria* / metabolism
  • Peptaibols* / pharmacology
  • Reactive Oxygen Species* / metabolism
  • Xenograft Model Antitumor Assays

Substances

  • Antineoplastic Agents
  • Reactive Oxygen Species
  • Peptaibols