Total synthesis of the taraxacine A natural product via Ag(I)-catalysed imidate-alkyne cyclization

Org Biomol Chem. 2024 Dec 24. doi: 10.1039/d4ob01876a. Online ahead of print.

Abstract

A domino approach towards β-carboline natural product taraxacine A and its analogues was developed. The main step relies on a silver(I) and base co-catalysed imidate-alkyne cyclization. The reaction tolerates primary and secondary alcohols, and various substitutions in the indole are possible.