Mechanism of connexin channel inhibition by mefloquine and 2-aminoethoxydiphenyl borate

PLoS One. 2024 Dec 31;19(12):e0315510. doi: 10.1371/journal.pone.0315510. eCollection 2024.

Abstract

Gap junction intercellular communication (GJIC) between two adjacent cells involves direct exchange of cytosolic ions and small molecules via connexin gap junction channels (GJCs). Connexin GJCs have emerged as drug targets, with small molecule connexin inhibitors considered a viable therapeutic strategy in several diseases. The molecular mechanisms of GJC inhibition by known small molecule connexin inhibitors remain unknown, preventing the development of more potent and connexin-specific therapeutics. Here we show that two GJC inhibitors, mefloquine (MFQ) and 2-aminoethoxydiphenyl borate (2APB) bind to Cx32 and block dye permeation across Cx32 hemichannels (HCs) and GJCs. Cryo-EM analysis shows that 2APB binds to "site A", close to the N-terminal gating helix of Cx32 GJC, restricting the entrance to the channel pore. In contrast, MFQ binds to a distinct "site M", deeply buried within the pore. MFQ binding to this site modifies the electrostatic properties of Cx32 pore. Mutagenesis of V37, a key residue located in the site M, renders Cx32 HCs and GJCs insensitive to MFQ-mediated inhibition. Moreover, our cryo-EM analysis, mutagenesis and activity assays show that MFQ targets the M site in Cx43 GJC similarly to Cx32. Taken together, our results point to a conserved inhibitor binding site in connexin channels, opening a new route for development of specific drugs targeting connexins.

MeSH terms

  • Animals
  • Binding Sites
  • Boron Compounds* / chemistry
  • Boron Compounds* / pharmacology
  • Cell Communication / drug effects
  • Connexins* / antagonists & inhibitors
  • Connexins* / chemistry
  • Connexins* / genetics
  • Connexins* / metabolism
  • Cryoelectron Microscopy
  • Gap Junction beta-1 Protein
  • Gap Junctions* / drug effects
  • Gap Junctions* / metabolism
  • Humans
  • Mefloquine* / pharmacology

Substances

  • Mefloquine
  • Connexins
  • Boron Compounds
  • 2-aminoethoxydiphenyl borate
  • Gap Junction beta-1 Protein

Grants and funding

The work was supported by the Swiss National Science Foundation (grant 184915) to V.M.K. the funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript.