CCR5-ligand decorated rilpivirine lipid-based nanoparticles for sustained antiretroviral responses

Nat Commun. 2025 Jan 8;16(1):513. doi: 10.1038/s41467-024-55544-9.

Abstract

Antiretroviral therapy (ART) improves the quality of life for those living with the human immunodeficiency virus type one (HIV-1). However, poor compliance reduces ART effectiveness and leads to immune compromise, viral mutations, and disease co-morbidities. Here we develop a drug formulation in which a lipid-based nanoparticle (LBNP) carrying rilpivirine (RPV) is decorated with the C-C chemokine receptor type 5 (CCR5) targeting peptide. This facilitates extended drug persistence within myeloid cells. Particle delivery to viral reservoirs is tracked by positron emission tomography. The CCR5-mediated LBNP cell uptake and retention reduce HIV-1 replication in human monocyte-derived macrophages and infected humanized mice (hu mice). Focused ultrasound with microbubbles mediated blood brain barrier (BBB) disruption allows the CCR5-targeted LBNP to penetrate the BBB and reach brain myeloid cells. These findings offer a role for CCR5-targeted therapeutics in antiretroviral delivery to optimize HIV suppression.

MeSH terms

  • Animals
  • Anti-HIV Agents / administration & dosage
  • Anti-HIV Agents / chemistry
  • Anti-HIV Agents / pharmacokinetics
  • Anti-HIV Agents / pharmacology
  • Blood-Brain Barrier* / drug effects
  • Blood-Brain Barrier* / metabolism
  • HIV Infections* / drug therapy
  • HIV Infections* / virology
  • HIV-1* / drug effects
  • Humans
  • Ligands
  • Lipids / chemistry
  • Liposomes
  • Macrophages / metabolism
  • Mice
  • Nanoparticles* / chemistry
  • Receptors, CCR5* / metabolism
  • Rilpivirine* / administration & dosage
  • Rilpivirine* / pharmacokinetics
  • Rilpivirine* / pharmacology
  • Virus Replication / drug effects

Substances

  • Rilpivirine
  • Receptors, CCR5
  • Anti-HIV Agents
  • CCR5 protein, human
  • Lipids
  • Ligands
  • Lipid Nanoparticles
  • Liposomes