Redox regulation of NF-kappa B DNA binding activity by dihydrolipoate

Biochem Mol Biol Int. 1995 Jun;36(2):241-6.

Abstract

NF-kappa B transcription factor regulates a wide variety of cellular and viral genes including the human immunodeficiency virus type 1. Here, we demonstrate that dihydrolipoate/alpha-lipoate redox couple which is a cofactor for mitochondrial dehydrogenases reactions, influences the DNA binding activity of NF-kappa B. The elimination of dithiothreitol in the electrophoretic mobility shift assay protocol resulted in the inability to detect DNA binding activity of activated NF-kappa B. The DNA binding activity was restored by the addition of dihydrolipoate in the binding reaction mixture. Inhibition of NF-kappa B DNA binding activity by in vitro exposure to a sulfhydryl oxidizing agent, diamide was also blocked by dihydrolipoate. In contrast, the addition of the oxidized form, alpha-lipoate inhibited the NF-kappa B DNA binding activity. Coincidentally, preincubation of Jurkat cells with dihydrolipoate potentiated and alpha-lipoate inhibited the okadaic acid-induced NF-kappa B activation as detected by assessing its DNA binding activity. These results suggest the redox exchange between lipoate and NF-kappa B molecules. Furthermore, since the inhibition of AP-1 DNA binding activity by diamide was also blocked by dihydrolipoate, this natural reductant may participate in the redox regulation of transcription factors by enhancing the DNA-protein interactions.

MeSH terms

  • Base Sequence
  • Cell Nucleus / metabolism
  • DNA / metabolism*
  • DNA Probes
  • Diamide / pharmacology
  • Dithiothreitol / pharmacology
  • Ethers, Cyclic / pharmacology
  • Humans
  • Molecular Sequence Data
  • NF-kappa B / metabolism*
  • Okadaic Acid
  • Oxidation-Reduction
  • Thioctic Acid / analogs & derivatives*
  • Thioctic Acid / metabolism
  • Thioctic Acid / pharmacology
  • Transcription Factor AP-1 / metabolism
  • Tumor Cells, Cultured
  • Tumor Necrosis Factor-alpha / pharmacology

Substances

  • DNA Probes
  • Ethers, Cyclic
  • NF-kappa B
  • Transcription Factor AP-1
  • Tumor Necrosis Factor-alpha
  • Diamide
  • Okadaic Acid
  • Thioctic Acid
  • dihydrolipoic acid
  • DNA
  • Dithiothreitol