Intracellular glutathione levels regulate Fos/Jun induction and activation of glutathione S-transferase gene expression

Cancer Res. 1994 Jan 1;54(1):36-40.

Abstract

Induction of glutathione S-transferase Ya and NAD(P)H:quinone reductase gene expression by a variety of chemical agents is mediated by regulatory elements, EpRE and ARE, composed of two adjacent AP-1-like binding sites and activated by Fos/Jun heterodimeric complex (AP-1). Recent studies show that chemical induction of glutathione S transferase Ya and quinone reductase gene expression is associated with an induction of c-fos and c-jun gene expression and AP-1 binding activity. In this report we present evidence that the AP-1 binding activity and the expression of chloramphenicol acetyltransferase activity from an EpRE Ya-cat gene construct are induced by an increase in intracellular oxidant levels. We observe that lowering the glutathione levels with buthionine sulfoximine, an inhibitor of gamma-glutamylcysteine synthetase, or diamide, a thiol-oxidizing agent, stimulates both basal and chemical-inducible expression of chloramphenicol acetyltransferase activity from EpRE Ya-cat and the AP-1 binding activity. Furthermore, we observe that the induction of these activities by a variety of chemical agents is inhibited by thiol compounds N-acetylcysteine and glutathione. These findings suggest that diverse chemicals that induce the AP-1 complex, leading to the AP-1-mediated transcriptional activation of glutathione S-transferase Ya gene expression, may act through a common mechanism involving the production of reactive oxygen species and depletion of reduced glutathione.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Buthionine Sulfoximine
  • Carcinoma, Hepatocellular / enzymology
  • Chloramphenicol O-Acetyltransferase / metabolism*
  • Diamide / pharmacology
  • Electron Spin Resonance Spectroscopy
  • Enzyme Induction / drug effects
  • Enzyme Induction / genetics
  • Gene Expression Regulation, Enzymologic / genetics*
  • Genes, fos / physiology
  • Genes, jun / physiology
  • Glutathione / physiology*
  • Glutathione Transferase / biosynthesis*
  • Glutathione Transferase / genetics
  • Humans
  • Methionine Sulfoximine / analogs & derivatives
  • Methionine Sulfoximine / pharmacology
  • Proto-Oncogene Proteins c-fos / metabolism
  • Proto-Oncogene Proteins c-fos / physiology*
  • Proto-Oncogene Proteins c-jun / metabolism
  • Proto-Oncogene Proteins c-jun / physiology*
  • Tumor Cells, Cultured

Substances

  • Proto-Oncogene Proteins c-fos
  • Proto-Oncogene Proteins c-jun
  • Diamide
  • Methionine Sulfoximine
  • Buthionine Sulfoximine
  • Chloramphenicol O-Acetyltransferase
  • Glutathione Transferase
  • Glutathione