Synthesis and biological properties of a biotinylated derivative of ACTH1-17 for MSH receptor studies

J Recept Res. 1993;13(1-4):229-44. doi: 10.3109/10799899309073657.

Abstract

A biotinylated derivative of [beta-Ala1,Lys17]-ACTH1-17-NH-(CH2)4-NH2 (ACTH1-17) was synthesized and biologically characterized. The heptadecapeptide with free N-terminus and blocked side-chains was prepared by the solid-phase method using TentaGel resin and a 4-aminobutylamide linker. Biotinyl-beta-Ala-OH was then coupled to the terminal amino group and the resulting [N alpha-(biotinyl-beta-alanyl)-beta-Ala1,Lys17]-ACTH1-17-NH-(CH2)4-N H2 (Bio-ACTH1-17) cleaved from the resin, purified and analyzed. Competition binding assays with mouse B16-F1 and human D10 and HBL melanoma cells using [125I]-alpha-MSH as radioligand gave dissociation constants for Bio-ACTH1-17 of 1.67 +/- 0.07 nM (B16-F1), 0.02 +/- 0.005 nM (D10) and 0.21 +/- 0.02 nM (HBL). The EC50 for Bio-ACTH1-17 in the B16 melanin assay was 4.15 +/- 1.0 nM. Analysis of the binding characteristics of [125I]-Bio-ACTH1-17 demonstrated that in human melanoma cells this radioligand was displaced by ACTH1-17 as well as alpha-MSH whereas in B16-F1 cells the tracer was only displaced from the binding site by ACTH1-17. Studies of Bio-ACTH1-17 with streptavidin showed that the peptide is to a large extent trapped specifically through reaction with biotin. These results demonstrate that (1) the biological characteristics of Bio-ACTH1-17 are almost identical to those of ACTH1-17, (2) Bio-ACTH1-17 is bound by avidin, and (3) Bio-ACTH1-17 may become a useful tool for MSH receptor targeting.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adrenocorticotropic Hormone / chemical synthesis*
  • Adrenocorticotropic Hormone / metabolism
  • Adrenocorticotropic Hormone / pharmacology
  • Amino Acid Sequence
  • Animals
  • Biological Assay
  • Biotin / analogs & derivatives*
  • Biotin / chemical synthesis
  • Biotin / metabolism
  • Biotin / pharmacology
  • Humans
  • Melanins / biosynthesis
  • Melanoma, Experimental / metabolism
  • Mice
  • Molecular Sequence Data
  • Peptide Fragments / chemical synthesis*
  • Peptide Fragments / metabolism
  • Peptide Fragments / pharmacology
  • Receptors, Pituitary Hormone / metabolism*
  • Sensitivity and Specificity
  • Tumor Cells, Cultured

Substances

  • ACTH (1-17)-NH-(CH2)4-NH2, (Nalpha-(biotinyl-beta-Ala(1))-Lys(17))-
  • Melanins
  • Peptide Fragments
  • Receptors, Pituitary Hormone
  • Biotin
  • MSH receptor
  • Adrenocorticotropic Hormone