Purification and characterization of a dipeptidase from Pseudomonas fluorescens ATCC 948

J Dairy Sci. 1996 Mar;79(3):357-65. doi: 10.3168/jds.S0022-0302(96)76372-5.

Abstract

A dipeptidase from a cell extract of Pseudomonas fluorescens ATCC 948 was purified to homogeneity by ion-exchange chromatography, hydroxyapatite chromatography, gel filtration, and FPLC Phenyl Superose chromatography. The enzyme was located in the cytoplasmic fraction. The dipeptidase appeared to be a monomer with a molecular mass of about 46 kDa, and activity was optimal at pH 8.0 and 50 degrees C. Although activity decreased markedly at temperatures > 50 degrees C, about 50% of maximal activity was retained at 10 degrees C. The activity was inhibited by EDTA, but could be reactivated with Co2+ and partially reactivated with Ca2+. Reducing agents, such as dithiothreitol and 8-hydroxyquinoline, also strongly inhibited the enzyme. The dipeptidase hydrolyzed only dipeptides and showed a particular aptitude for substrates containing a hydrophobic AA at the N-terminus. Dipeptides containing a proline residue were not cleaved. Kinetic studies indicated that the dipeptidase hydrolyzed Leu-Leu with a Michaelis-Menten constant of 0.43 mM and a turnover number of 1812/s.

MeSH terms

  • Calcium / pharmacology
  • Chromatography
  • Chromatography, Gel
  • Chromatography, High Pressure Liquid
  • Chromatography, Ion Exchange
  • Cobalt / pharmacology
  • Dipeptidases / chemistry
  • Dipeptidases / isolation & purification*
  • Dipeptidases / metabolism
  • Dithiothreitol / pharmacology
  • Edetic Acid / pharmacology
  • Enzyme Inhibitors / pharmacology
  • Hydrogen-Ion Concentration
  • Kinetics
  • Molecular Weight
  • Oxyquinoline / pharmacology
  • Pseudomonas fluorescens / enzymology*
  • Substrate Specificity
  • Sulfhydryl Reagents / pharmacology

Substances

  • Enzyme Inhibitors
  • Sulfhydryl Reagents
  • Cobalt
  • Oxyquinoline
  • Edetic Acid
  • Dipeptidases
  • dipeptidase
  • Calcium
  • Dithiothreitol