Biochemical characterisation of ketoconazole inhibitory action on Aspergillus fumigatus

FEMS Immunol Med Microbiol. 1996 Nov;16(1):11-20. doi: 10.1111/j.1574-695X.1996.tb00106.x.

Abstract

The effect of ketoconazole on growth, sterol composition, in vitro sterol biosynthesis and P450-CO complex formation and its interaction with microsomal P450 was determined. On solid medium and in liquid medium ketoconazole inhibited Aspergillus fumigatus growth completely at 5 x 10(-5) M and 50% of the growth at 1.3 x 10(-5) M and 2.1 x 10(-5) M respectively. A close relationship between accumulation of 14 alpha-methyl sterols (eburicol, obtusifoliol and 14 alpha-methyl fecosterol) and depletion of ergosterol with growth arrest was observed in ketoconazole treated cultures. The half inhibitory concentration for in vitro ergosterol biosynthesis and half saturating concentration for type II binding spectrum of ketoconazole were calculated as 73.8 +/- 6.3 nM and 0.13 +/- 0.04 microM respectively. CO displacement studies revealed inhibition of CO-P450 complex formation by ketoconazole.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antifungal Agents / administration & dosage
  • Antifungal Agents / pharmacology*
  • Aspergillus fumigatus / drug effects*
  • Aspergillus fumigatus / growth & development
  • Aspergillus fumigatus / metabolism
  • Carbon Monoxide / metabolism
  • Chromatography, Gas
  • Cytochrome P-450 Enzyme System / metabolism
  • Ketoconazole / administration & dosage
  • Ketoconazole / pharmacology*
  • Mass Spectrometry
  • Microsomes / metabolism
  • Molecular Structure
  • Sterols / biosynthesis
  • Sterols / metabolism
  • Time Factors

Substances

  • Antifungal Agents
  • Sterols
  • Carbon Monoxide
  • Cytochrome P-450 Enzyme System
  • Ketoconazole