Simultaneous analysis of retinol, all-trans- and 13-cis-retinoic acid and 13-cis-4-oxoretinoic acid in plasma by liquid chromatography using on-column concentration after single-phase fluid extraction

J Chromatogr B Biomed Sci Appl. 1997 Jun 20;694(1):83-92. doi: 10.1016/s0378-4347(97)00109-6.

Abstract

A reversed-phase high-performance liquid chromatographic method for the simultaneous analysis of retinol, all-trans-retinoic acid, 13-cis-retinoic acid and 13-cis-4-oxoretinoic acid in human plasma and cell culture medium is described. Sample preparation involves precipitation of proteins and extraction of retinoids with 60% acetonitrile. After centrifugation, the acetonitrile content of the supernatant is reduced to 45%, allowing on-column concentration of analytes. Injection volumes up to 2.0 ml (equivalent to 0.525 ml of sample) can be used without compromising chromatographic resolution of all-trans-retinoic acid and 13-cis-retinoic acid. Retinoids were stable in this extract and showed no isomerization when stored in the dark in a cooled autosampler, allowing automated analysis of large series of samples. Recoveries from spiked plasma samples were between 95 and 103%. Although no internal standard was used, the inter-assay precision for all retinoids was better than 6% and 4% at concentrations of 30 nM and 100 nM, respectively. The method is a valuable tool for the study of cellular metabolism of all-trans-retinoic acid, as polar metabolites of this compound can be detected with high sensitivity in cell culture media.

MeSH terms

  • Chromatography, High Pressure Liquid
  • Drug Stability
  • Humans
  • Isotretinoin / blood*
  • Solubility
  • Tretinoin / analogs & derivatives*
  • Tretinoin / blood*
  • Tretinoin / metabolism
  • Tumor Cells, Cultured
  • Vitamin A / blood*

Substances

  • Vitamin A
  • 4-oxoretinoic acid
  • Tretinoin
  • Isotretinoin