New botrydial sesquiterpenoids from Hymenoscyphus epiphyllus

Z Naturforsch C J Biosci. 1997 Jul-Aug;52(7-8):413-20. doi: 10.1515/znc-1997-7-801.

Abstract

Four new botrydial derivatives, hymendial (1), 7 alpha-hydroxydihydrobotrydial (2), 7 alpha-hydroxy-10-O-methyldihydrobotrydial (4), and 7 alpha-acetoxy-15 alpha-methoxy-10-O-methyl-dihydrobotrydial (5) were isolated together with dihydrobotrydial (3) from the culture fluid of the ascomycete Hymenoscyphus epiphyllus. In addition, cytochalasin H (6a), 18-deoxycytochalasin H (6b) and (+)-mellein (7) were produced by this fungus. Hymendial (1), possessing an alpha, beta-unsaturated dialdehyde functionality, exhibits antimicrobial and cytotoxic activities and is mutagenic in the Ames Salmonella assay.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Antineoplastic Agents / chemistry*
  • Antineoplastic Agents / isolation & purification
  • Antineoplastic Agents / toxicity
  • Ascomycota / chemistry*
  • Ascomycota / growth & development
  • Cell Line
  • Cell Survival / drug effects*
  • Fermentation
  • HeLa Cells
  • Humans
  • Leukemia L1210
  • Mice
  • Microbial Sensitivity Tests
  • Molecular Structure
  • Nuclear Magnetic Resonance, Biomolecular
  • Salmonella typhimurium / drug effects
  • Sesquiterpenes / chemistry*
  • Sesquiterpenes / isolation & purification
  • Sesquiterpenes / pharmacology
  • Tumor Cells, Cultured

Substances

  • Antineoplastic Agents
  • Sesquiterpenes