Substitution of Arg-244 by Cys or Ser in SHV-1 and SHV-5 beta-lactamases confers resistance to mechanism-based inhibitors and reduces catalytic efficiency of the enzymes

FEMS Microbiol Lett. 1998 Mar 1;160(1):49-54. doi: 10.1111/j.1574-6968.1998.tb12889.x.

Abstract

The conserved residue Arg-244 was substituted by the smaller uncharged amino acids Cys and Ser in SHV-1 and SHV-5 beta-lactamases by a PCR-based site-specific mutagenesis procedure. The mutant beta-lactamases displayed decreased susceptibility to clavulanate and, to a lesser extent, to tazobactam and sulbactam. As shown in comparative MIC determinations, R244C and R244S enzymes retained a residual penicillinase activity while their activity towards cephalosporins was drastically diminished. The respective SHV-5 mutants were unable to hydrolyze oxyimino-beta-lactams except aztreonam. The impaired catalytic activity of the mutant beta-lactamases was mainly due to the lowering of affinity for beta-lactam substrates. The above alterations were more pronounced in the R244C mutants. These results provide information on the mode of involvement of Arg-244 in (a) inactivation by beta-lactamase inhibitors and (b) the proper positioning of beta-lactams in the active site of SHV enzymes.

MeSH terms

  • Amino Acid Substitution*
  • Anti-Bacterial Agents
  • Arginine
  • Clavulanic Acid
  • Cloning, Molecular
  • Cysteine
  • Escherichia coli / drug effects
  • Escherichia coli / enzymology*
  • Escherichia coli / genetics*
  • Microbial Sensitivity Tests
  • Penicillin Resistance
  • Serine
  • beta-Lactamases / genetics*

Substances

  • Anti-Bacterial Agents
  • Clavulanic Acid
  • Serine
  • Arginine
  • beta-lactamase PIT-2
  • beta-lactamase SHV-5
  • beta-Lactamases
  • Cysteine