Binding characteristics of a potent AMPA receptor antagonist [3H]Ro 48-8587 in rat brain

J Neurochem. 1998 Jul;71(1):418-26. doi: 10.1046/j.1471-4159.1998.71010418.x.

Abstract

A new AMPA receptor antagonist, Ro 48-8587, was characterized pharmacologically in vitro. It is highly potent and selective for AMPA receptors as shown by its effects on [3H]AMPA, [3H] kainate, and [3H] MK-801 binding to rat brain membranes and on AMPA- or NMDA-induced depolarization in rat cortical wedges. [3H]Ro 48-8587 bound with a high affinity (KD = 3 nM) to a single population of binding sites with a Bmax of 1 pmol/mg of protein in rat whole brain membranes. [3H]Ro 48-8587 binding to rat whole brain membranes was inhibited by several compounds with the following rank order of potency: Ro 48-8587 > 6-nitro-7-sulphamoylbenzo[f] quinoxaline-2,3-dione (NBQX) > YM 90K > 6-cyano-7-nitroquinoxaline-2,3-dione (CNQX) > quisqualate > AMPA > glutamate > kainate > NMDA. The distribution and abundance of specific binding sites (approximately 95% of total) in sections of rat CNS, revealed by quantitative receptor radioautography and image analysis, indicated a very discrete localization. Highest binding values were observed in cortical layers (binding in layers 1 and 2 > binding in layers 3-6), hippocampal formation, striatum, dorsal septum, reticular thalamic nucleus, cerebellar molecular layer, and spinal cord dorsal horn. At 1 nM, the values for specific binding were highest in the cortical layers 1 and 2 and lowest in the brainstem (approximately 2.6 and 0.4 pmol/mg of protein, respectively). Ro 48-8587 is a potent and selective AMPA receptor antagonist with improved binding characteristics (higher affinity, selectivity, and specific binding) compared with those previously reported.

MeSH terms

  • Animals
  • Anti-Anxiety Agents*
  • Benzodiazepines / pharmacology
  • Brain Chemistry*
  • Dizocilpine Maleate / metabolism
  • Dizocilpine Maleate / pharmacology
  • Electrophysiology
  • Excitatory Amino Acid Agonists / metabolism
  • Excitatory Amino Acid Agonists / pharmacology
  • Excitatory Amino Acid Antagonists / metabolism
  • Excitatory Amino Acid Antagonists / pharmacology*
  • Imidazoles / metabolism
  • Imidazoles / pharmacology*
  • In Situ Hybridization
  • Kainic Acid / metabolism
  • Kainic Acid / pharmacology
  • Kinetics
  • Male
  • N-Methylaspartate / metabolism
  • N-Methylaspartate / pharmacology
  • Quinazolines / metabolism
  • Quinazolines / pharmacology*
  • Quinoxalines / pharmacology
  • RNA, Messenger / analysis
  • Radioligand Assay
  • Rats
  • Rats, Inbred Strains
  • Receptors, AMPA / agonists
  • Receptors, AMPA / antagonists & inhibitors*
  • Receptors, AMPA / genetics*
  • Tritium
  • alpha-Amino-3-hydroxy-5-methyl-4-isoxazolepropionic Acid / metabolism
  • alpha-Amino-3-hydroxy-5-methyl-4-isoxazolepropionic Acid / pharmacology

Substances

  • Anti-Anxiety Agents
  • Excitatory Amino Acid Agonists
  • Excitatory Amino Acid Antagonists
  • Imidazoles
  • Quinazolines
  • Quinoxalines
  • RNA, Messenger
  • Receptors, AMPA
  • Ro 48-8587
  • Tritium
  • GYKI 52466
  • 2,3-dioxo-6-nitro-7-sulfamoylbenzo(f)quinoxaline
  • Benzodiazepines
  • 6-(1H-imidazol-1-yl)-7-nitro-2,3(1H,4H)-quinoxalinedione
  • N-Methylaspartate
  • Dizocilpine Maleate
  • alpha-Amino-3-hydroxy-5-methyl-4-isoxazolepropionic Acid
  • Kainic Acid