Metabolic studies on BMS-200475, a new antiviral compound active against hepatitis B virus

Antimicrob Agents Chemother. 1999 Jan;43(1):190-3. doi: 10.1128/AAC.43.1.190.

Abstract

BMS-200475 was recently shown to have potent antiviral activity against hepatitis B virus (50% effective concentration = 3.7 nM; 50% cytotoxic concentration = 30 microM). In metabolic studies in both HepG2 and hepatitis B virus-transfected 2.2.15 human hepatoma cell lines, the metabolism was similar, the primary products being the di- and triphosphates. The accumulation of triphosphate was rapid and detectable down to a 5 nM concentration of added drug. When cells were labeled at 25 microM, the intracellular triphosphate concentration attained 30 pmol/10(6) cells ( approximately 30 microM). The intracellular half-life of the triphosphate was about 15 h. Compared with five other nucleoside analogs of medical interest (lamivudine, penciclovir, ganciclovir, acyclovir, and lobucavir), BMS-200475 was most efficiently phosphorylated to the triphosphate in HepG2 cells.

MeSH terms

  • Antiviral Agents / metabolism*
  • Antiviral Agents / pharmacology
  • Deoxyguanosine / analogs & derivatives*
  • Deoxyguanosine / metabolism
  • Deoxyguanosine / pharmacology
  • Half-Life
  • Hepatitis B virus / drug effects
  • Hepatitis B virus / metabolism*
  • Humans
  • Phosphorylation
  • Spectrophotometry, Ultraviolet
  • Transfection
  • Tumor Cells, Cultured

Substances

  • Antiviral Agents
  • entecavir
  • Deoxyguanosine