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Characterization of surface organometallic complexes using high resolution 2D solid-state NMR spectroscopy. Application to the full characterization of a silica supported metal carbyne: (triple bond)SiO-Mo((triple bond)C-Bu-t)(CH(2)-Bu-t)(2).
Saint-Arroman RP, Chabanas M, Baudouin A, Copéret C, Basset JM, Lesage A, Emsley L. Saint-Arroman RP, et al. Among authors: chabanas m. J Am Chem Soc. 2001 Apr 25;123(16):3820-1. doi: 10.1021/ja002259n. J Am Chem Soc. 2001. PMID: 11457115 No abstract available.
Detailed structural investigation of the grafting of [Ta(=CHtBu)(CH2tBu)3] and [Cp*TaMe4] on silica partially dehydroxylated at 700 degrees C and the activity of the grafted complexes toward alkane metathesis.
Le Roux E, Chabanas M, Baudouin A, de Mallmann A, Copéret C, Quadrelli EA, Thivolle-Cazat J, Basset JM, Lukens W, Lesage A, Emsley L, Sunley GJ. Le Roux E, et al. Among authors: chabanas m. J Am Chem Soc. 2004 Oct 20;126(41):13391-9. doi: 10.1021/ja046486r. J Am Chem Soc. 2004. PMID: 15479095
Molecular Insight Into Surface Organometallic Chemistry Through the Combined Use of 2D HETCOR Solid-State NMR Spectroscopy and Silsesquioxane Analogues We are also indebted to the CNRS, ENS Lyon, and ESCPE Lyon for financial support. M.C. is grateful to the French ministry of education, research, and technology (MENRT) for a pre-doctoral fellowship. E.A.Q. gratefully acknowledges Università di Pisa and S.N.A.M. for financial support. 2D HETCOR=two-dimensional heteronuclear correlation.
Chabanas M, Quadrelli EA, Fenet B, Copéret C, Thivolle-Cazat J, Basset JM, Lesage A, Emsley L. Chabanas M, et al. Angew Chem Int Ed Engl. 2001 Dec 3;40(23):4493-4496. doi: 10.1002/1521-3773(20011203)40:23<4493::aid-anie4493>3.0.co;2-x. Angew Chem Int Ed Engl. 2001. PMID: 12404457 No abstract available.
Beta-H transfer from the metallacyclobutane: a key step in the deactivation and byproduct formation for the well-defined silica-supported rhenium alkylidene alkene metathesis catalyst.
Leduc AM, Salameh A, Soulivong D, Chabanas M, Basset JM, Copéret C, Solans-Monfort X, Clot E, Eisenstein O, Böhm VP, Röper M. Leduc AM, et al. Among authors: chabanas m. J Am Chem Soc. 2008 May 14;130(19):6288-97. doi: 10.1021/ja800189a. Epub 2008 Apr 11. J Am Chem Soc. 2008. PMID: 18402448
Low-Temperature Hydrogenolysis of Alkanes Catalyzed by a Silica-Supported Tantalum Hydride Complex, and Evidence for a Mechanistic Switch from Group IV to Group V Metal Surface Hydride Complexes We are grateful to Dr. L. Lefort, Dr. O. Maury (LCOMS), Dr. C. Meric de Bellefon, and Dr. D. Schweich from the laboratory LGPC (ESCPE Lyon) for fruitful discussions. We wish to thank the CNRS, and the ESCPE-Lyon for financial support. M.C. is also grateful to the French Ministry for Education, Research, and Technology (MENRT) for a predoctoral fellowship.
Chabanas M, Vidal V V, Copéret C, Thivolle-Cazat J, Basset JM. Chabanas M, et al. Angew Chem Int Ed Engl. 2000 Jun 2;39(11):1962-1965. doi: 10.1002/1521-3773(20000602)39:11<1962::aid-anie1962>3.0.co;2-1. Angew Chem Int Ed Engl. 2000. PMID: 10940996 No abstract available.
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