Abstract
Ising kagome antiferromagnets (KAFs) are rare in reality. In this paper, we report the magnetic ground state and field-induced transitions of an Ising antiferromagnet with a stacked kagome geometry, . Upon cooling, magnetic susceptibility measurements reveal three successive magnetic transitions at = 45.2 K, = 35.4 K, and 20 K. When the magnetic field is applied along the Ising axis, a strikingly anomalous initial magnetization lying outside the hysteresis loop is observed below . Through detailed characterizations, the magnetic field vs temperature phase diagram is established. A partially disordered antiferromagnetic state is proposed below , which becomes frozen below . is therefore a promising candidate for Ising KAFs, and this unique composite structure may shed light on the exploratory path for Ising KAFs.
2 More- Received 7 December 2021
- Accepted 29 March 2022
DOI:https://doi.org/10.1103/PhysRevB.105.144406
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