Backbone dynamics of the channel-forming antibiotic zervamicin IIB studied by 15N NMR relaxation

FEBS Lett. 2001 Apr 20;495(1-2):52-5. doi: 10.1016/s0014-5793(01)02363-8.

Abstract

The backbone dynamics of the channel-forming peptide antibiotic zervamicin IIB (Zrv-IIB) in methanol were studied by 15N nuclear magnetic resonance relaxation measurements at 11.7, 14.1 and 18.8 T magnetic fields. The anisotropic overall rotation of the peptide was characterized based on 15N relaxation data and by hydrodynamic calculations. 'Model-free' analysis of the relaxation data showed that the peptide is fairly rigid on a sub-nanosecond time-scale. The residues from the polar side of Zrv-IIB helix are involved in micro-millisecond time-scale conformational exchange. The conformational exchange observed might indicate intramolecular processes or specific intermolecular interactions of potential relevance to Zrv-IIB ion channel formation.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Anisotropy
  • Anti-Bacterial Agents / chemistry*
  • Computer Simulation
  • Ion Channels / chemistry*
  • Methanol / chemistry
  • Molecular Conformation
  • Nitrogen Isotopes
  • Nuclear Magnetic Resonance, Biomolecular*
  • Peptaibols
  • Peptides*
  • Rotation

Substances

  • Anti-Bacterial Agents
  • Ion Channels
  • Nitrogen Isotopes
  • Peptaibols
  • Peptides
  • zervamicin IIB
  • Methanol