Routine quality control of recycled target [18O]water by capillary electrophoresis and gas chromatography

Nucl Med Biol. 2003 Oct;30(7):785-90. doi: 10.1016/s0969-8051(03)00083-0.

Abstract

Recycling of [(18)O]water for [(18)F]fluoride production can be accomplished with reliable results. We have developed sensitive, robust, and rapid analyses of impurities in [(18)O]water. Anions were quantitated by capillary electrophoresis and organic residuals were quantitated by gas chromatography using methods with excellent reproducibility and linearity. Kryptofix 222 (K-222) was quantitated by a sensitive LC-MS-MS technique. Isotopic composition was determined by GC-MS with satisfactory accuracy and precision. These methods were employed to evaluate recovered [(18)O]water purified by a novel electrolysis method. 2-[(18)F]FDG yields using purified [(18)O]water with very low levels of impurities are indistinguishable from newly purchased [(18)O]water. High (> 300 ppm) carbonate concentration reduces the fluoride trapping efficiency of QMA. The analyses of anions, organics, and isotopic enrichment were applied routinely for quality control of [(18)O]water to predict a satisfactory outcome of 2-[(18)F]FDG production.

Publication types

  • Comparative Study
  • Evaluation Study
  • Validation Study

MeSH terms

  • Chromatography, Gas / methods*
  • Conservation of Natural Resources / methods
  • Drug Stability
  • Electrophoresis, Capillary / methods*
  • Fluorodeoxyglucose F18 / chemical synthesis*
  • Fluorodeoxyglucose F18 / isolation & purification*
  • Fluorodeoxyglucose F18 / standards
  • Oxygen Isotopes / chemistry*
  • Oxygen Isotopes / isolation & purification*
  • Oxygen Isotopes / standards
  • Quality Control
  • Radiopharmaceuticals / chemistry
  • Radiopharmaceuticals / isolation & purification
  • Radiopharmaceuticals / standards
  • Water / analysis
  • Water / chemistry*
  • Water / standards
  • Water Purification / methods*
  • Water Purification / standards

Substances

  • Oxygen Isotopes
  • Radiopharmaceuticals
  • Water
  • Fluorodeoxyglucose F18