Transforming bivalent ligands into retractable enzyme inhibitors through polypeptide-protein interactions

Bioorg Med Chem Lett. 2005 Dec 1;15(23):5120-3. doi: 10.1016/j.bmcl.2005.08.085. Epub 2005 Oct 3.

Abstract

The concept of bivalent polypeptides with controllable flexible linkers is demonstrated through the design of a new generation of 'antidote'-reversible inhibitors of thrombin. These molecules contain two binding moieties, each of which in isolation has only a moderate affinity of binding, which are linked together by a flexible peptide bridge. We show that activities of the potent bivalent inhibitors of thrombin can be reversed by the specific, but much weaker, binding of the linker moiety to protein 'antidotes'.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Humans
  • Ligands
  • Molecular Sequence Data
  • Peptides / chemistry
  • Peptides / pharmacology
  • Proteins / chemistry
  • Proteins / pharmacology
  • Serine Proteinase Inhibitors / chemistry*
  • Serine Proteinase Inhibitors / pharmacology
  • Thrombin / antagonists & inhibitors*

Substances

  • Ligands
  • Peptides
  • Proteins
  • Serine Proteinase Inhibitors
  • Thrombin