Nonadiabatic effects in resonant inelastic x-ray scattering

Phys Rev Lett. 2005 Oct 14;95(16):163002. doi: 10.1103/PhysRevLett.95.163002. Epub 2005 Oct 10.

Abstract

We have studied the spectral features of resonant inelastic x-ray scattering of condensed ethylene with vibrational selectivity both experimentally and theoretically. Purely vibrational spectral loss features and coupled electronic and vibrational losses are observed. The one-step theory for resonant soft x-ray scattering is applied, taking multiple vibrational modes and vibronic coupling into account. Our investigation of ethylene underlines that the assignment of spectral features observed in resonant inelastic x-ray scattering of polyatomic systems requires an explicit description of the coupled electronic and vibrational loss features.