Hirsutenone inhibits phorbol ester-induced upregulation of COX-2 and MMP-9 in cultured human mammary epithelial cells: NF-kappaB as a potential molecular target

FEBS Lett. 2006 Jan 23;580(2):385-92. doi: 10.1016/j.febslet.2005.12.015. Epub 2005 Dec 19.

Abstract

Inappropriate upregulation of cyclooxygenase-2 (COX-2) and matrix metalloproteinases (MMPs) has been implicated in the pathogenesis of various types of cancer. In the present study, we investigated the effects of hirsutenone, a diarylheptanoid isolated from the medicinal plant Alnus hirsuta var. sibirica, on the expression of COX-2 and MMP-9 induced by the tumor promoter 12-O-tetradecanoylphorbol-13-acetate (TPA) in MCF10A human breast epithelial cells. Treatment of MCF10A cells with TPA led to the expression of COX-2 and MMP-9. Hirsutenone at 12 microM inhibited the TPA-induced COX-2 expression at both the transcriptional and posttranscriptional levels. Hirsutenone also suppressed the synthesis of prostaglandin E(2), one of the major products of COX-2, and its catalytic activity. The upregulation of MMP-9 by TPA was also significantly reduced by hirsutenone. Likewise, hirsutenone attenuated the invasiveness and motility of MCF10A cells stimulated with TPA. Hirsutenone blocked the TPA-induced DNA binding of nuclear factor kappa B (NF-kappaB) and translocation of p65, the functionally active NF-kappaB subunit, to the nucleus. The luciferase reporter gene assay revealed that hirsutenone abrogated the transcriptional activity of NF-kappaB. Treatment of MCF10A cells with N-alpha-Tosyl-l-phenylalanine chloromethyl ketone, a specific inhibitor of NF-kappaB, reduced the TPA-induced expression of COX-2 and MMP-9. In summary, hirsutenone inhibits the TPA-induced upregulation of COX-2 and MMP-9 in human breast epithelial cells, possibly by targeting NF-kappaB, which may contribute to its chemopreventive effects.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Active Transport, Cell Nucleus / physiology
  • Catechols / pharmacology*
  • Cell Line
  • Cell Movement / physiology
  • Cyclooxygenase 2 / metabolism*
  • Diarylheptanoids / pharmacology*
  • Dinoprostone / biosynthesis
  • Epithelial Cells / cytology
  • Epithelial Cells / metabolism*
  • Gene Expression Regulation, Enzymologic
  • Genes, Reporter
  • Humans
  • Mammary Glands, Human / cytology*
  • Matrix Metalloproteinase 9 / metabolism*
  • Membrane Proteins / metabolism*
  • Molecular Structure
  • NF-kappa B / metabolism*
  • Tetradecanoylphorbol Acetate / metabolism*
  • Transcription, Genetic
  • Up-Regulation

Substances

  • Catechols
  • Diarylheptanoids
  • Membrane Proteins
  • NF-kappa B
  • hirsutenone
  • Cyclooxygenase 2
  • PTGS2 protein, human
  • Matrix Metalloproteinase 9
  • Dinoprostone
  • Tetradecanoylphorbol Acetate