Peroxynitrite induced formation of the neurotoxins 5-S-cysteinyl-dopamine and DHBT-1: implications for Parkinson's disease and protection by polyphenols

Arch Biochem Biophys. 2008 Aug 15;476(2):145-51. doi: 10.1016/j.abb.2008.03.011. Epub 2008 Mar 22.

Abstract

Mechanisms of nigral cell injury in Parkinson's disease remain unclear, although a combination of increased oxidative stress, the formation of catecholamine-quinones and the subsequent formation of neurotoxic cysteinyl-catecholamine conjugates may contribute. In the present study, peroxynitrite was observed to generate both 2-S- and 5-S-cysteinyl-dopamine and a dihydrobenzothiazine species, DHBT-1, following the reaction of dopamine with l-cysteine. The formation of 5-S-cysteinyl-dopamine and DHBT-1 in the presence of peroxynitrite induced significant neuronal injury. Pre-treatment of cortical neurons with pelargonidin, quercetin, hesperetin, caffeic acid, the 4'-O-Me derivatives of catechin and epicatechin (0.1-3.0 microM) resulted in concentration dependant protection against 5-S-cysteinyl-dopamine-induced neurotoxicity. These data suggest that polyphenols may protect against neuronal injury induced by endogenous neurotoxins relevant to the aetiology of the Parkinson disease.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Cell Culture Techniques
  • Cell Survival / drug effects
  • Cells, Cultured
  • Cerebral Cortex / cytology
  • Culture Media, Serum-Free
  • Dopamine / biosynthesis*
  • Dopamine / chemistry
  • Flavonoids / chemistry*
  • Flavonoids / pharmacology
  • Mice
  • Molecular Structure
  • Neurons / drug effects
  • Parkinson Disease / etiology*
  • Peroxynitrous Acid / pharmacology*
  • Phenols / chemistry*
  • Phenols / pharmacology
  • Polyphenols
  • Time Factors
  • Tryptamines / biosynthesis*
  • Tryptamines / chemistry

Substances

  • Culture Media, Serum-Free
  • Flavonoids
  • Phenols
  • Polyphenols
  • Tryptamines
  • 5,5'-dihydroxy-4,4'-bitryptamine
  • Peroxynitrous Acid
  • Dopamine